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DESCRIPTION:Neutron Scattering Investigations of Three-Dimensional Topological States\n\nMagnetic skyrmions represent a unique class of topological magnet characterized by nanometric swirling spin-textures which possess a non-trivial Berry curvature. The combination of their topological stability\, unique transport properties\, and emergent dynamics has made skyrmions the forerunner for novel spintronic high-density memory and ultra-low power logic device applications. In this thesis\, we explore the development and application of various neutron scattering tomography and structured neutron beam techniques for three-dimensional investigations of bulk magnetic topological materials and their defect-mediated dynamical phenomena. Characterization of the disordered multi-phase bulk skyrmion material\, Co8Zn8Mn4\, was performed through detailed SANS measurements over the entire temperature-magnetic field phase diagram of the material as a function of a dynamic skyrmion ordering sequence. 2D SANS images in combination with micromagnetic simulations reveal a novel disordered-to-ordered skyrmion square lattice transition pathway which represents a new type of non-charge conserving topological transition. In the metastable skyrmion triangular lattice phase\, dynamical field-dependent skyrmion responses showed an exotic memory phase in spite of hysteresis protocols involving field-induced saturation into the ferromagnetic phase. Three-dimensional examinations of skyrmion stabilization mechanisms and their dynamical defect pathways were explored using a novel SANS tomography technique which processes multi-projection neutron scattering images as its input. Application of the technique to the ordered thermal equilibrium skyrmion triangular lattice phase yielded the first three-dimensional visualizations of a bulk skyrmion lattice. The reconstructions unveiled a host of exotic skyrmion features\, such as branching\, segmented\, twisting\, and filament structures\, mediated by three-dimensional topological transitions through two different emergent monopole (MP)-antimonopole (AMP) defect pathways. Finally\, the direct identification and determination of topological features and defects in bulk micromagnetic materials\, without a priori knowledge of the sample\, was explored using holographic approaches for the generation of neutron helical waves. Linear neutron waves in a conventional SANS setup were input on microfabricated gratings which consist of arrays of various q-fold fork-dislocation phase-gratings with nanometric spatial dimensions. Far-field scattering images exhibited doughnut intensity profiles centered on the first diffraction orders\, thereby demonstrating the tunable generation of topological neutron states for phase- and topology-matched studies of quantum materials. The amalgamation of these works demonstrates the development and application of novel tools for direct investigations of bulk topological magnetic materials\, while uncovering a diverse collection of skyrmion energetics\, disorder-dependent dynamics\, and three-dimensional topological transition defect pathways. These methods and results open the door to a new generation of neutron scattering techniques for the probing of exotic topological interactions and the complete standalone characterization of quantum materials and their topological phenomena.\n 
X-ALT-DESC;FMTTYPE=text/html:<strong>Neutron Scattering Investigations of Three-Dimensional Topological States</strong><br><br>Magnetic skyrmions represent a unique class of topological magnet characterized by nanometric swirling spin-textures which possess a non-trivial Berry curvature. The combination of their topological stability, unique transport properties, and emergent dynamics has made skyrmions the forerunner for novel spintronic high-density memory and ultra-low power logic device applications. In this thesis, we explore the development and application of various neutron scattering tomography and structured neutron beam techniques for three-dimensional investigations of bulk magnetic topological materials and their defect-mediated dynamical phenomena. Characterization of the disordered multi-phase bulk skyrmion material, Co8Zn8Mn4, was performed through detailed SANS measurements over the entire temperature-magnetic field phase diagram of the material as a function of a dynamic skyrmion ordering sequence. 2D SANS images in combination with micromagnetic simulations reveal a novel disordered-to-ordered skyrmion square lattice transition pathway which represents a new type of non-charge conserving topological transition. In the metastable skyrmion triangular lattice phase, dynamical field-dependent skyrmion responses showed an exotic memory phase in spite of hysteresis protocols involving field-induced saturation into the ferromagnetic phase. Three-dimensional examinations of skyrmion stabilization mechanisms and their dynamical defect pathways were explored using a novel SANS tomography technique which processes multi-projection neutron scattering images as its input. Application of the technique to the ordered thermal equilibrium skyrmion triangular lattice phase yielded the first three-dimensional visualizations of a bulk skyrmion lattice. The reconstructions unveiled a host of exotic skyrmion features, such as branching, segmented, twisting, and filament structures, mediated by three-dimensional topological transitions through two different emergent monopole (MP)-antimonopole (AMP) defect pathways. Finally, the direct identification and determination of topological features and defects in bulk micromagnetic materials, without a priori knowledge of the sample, was explored using holographic approaches for the generation of neutron helical waves. Linear neutron waves in a conventional SANS setup were input on microfabricated gratings which consist of arrays of various q-fold fork-dislocation phase-gratings with nanometric spatial dimensions. Far-field scattering images exhibited doughnut intensity profiles centered on the first diffraction orders, thereby demonstrating the tunable generation of topological neutron states for phase- and topology-matched studies of quantum materials. The amalgamation of these works demonstrates the development and application of novel tools for direct investigations of bulk topological magnetic materials, while uncovering a diverse collection of skyrmion energetics, disorder-dependent dynamics, and three-dimensional topological transition defect pathways. These methods and results open the door to a new generation of neutron scattering techniques for the probing of exotic topological interactions and the complete standalone characterization of quantum materials and their topological phenomena.<strong><br /> </strong>
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SUMMARY:Melissa Henderson PhD Denfence
DTSTART;TZID=America/New_York:20231026T140000
DTEND;TZID=America/New_York:20231026T150000
DTSTAMP:20260420T033551Z
TRANSP:OPAQUE
STATUS:CONFIRMED
SEQUENCE:0
LOCATION:PHY 352
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